Kris wrote: Or are chords simply not applicable in these cases?
This might be true, Kris. At least, from what I remember from second year theory when we were analyzing the music of Schoenberg. We were just looking for permutations of the "tone rows" and didn't talk about chords at all. In that kind of atonal music, you wouldn't find the chord A-C-E anyway. It just wouldn't fit.
Interestingly, in "Romantic" music you might find traditional chords all over the place, but no "key center".
In first year theory, we learned how to analyze (I just now noticed that word has "anal" in it!

) baroque and classical music, mostly using the Bach part writing rules. In second year theory, on the first day our teacher gave us a piano reduction of
Liebestod from Richard Wagner's
Tristan und Isolde. He simply told us to take it home and analyze it. (Now I can't keep from laughing when I write that word).
The next day he asked, "What key is it in?" Nobody had an answer! While it uses standard chords, the key center keeps shifting so that you don't know WHERE you are anymore. The lesson was, that what makes Romantic music romantic is that feeling of being "lost". You never get what you expect to get. Sort of like the carrot on the end of the stick.
I know that doesn't answer your questions, but I found it very interesting and thought you might, too.
Alan